Let me try to answer your by addressing different scenarios.
1. For Spirited driving- If you are someone who loves to drive this vehicle in a spirited or enthisiastic way, then I would suggest you to go for Michelin Latitude Sport 3 tyre. It would offer superb high speed control and improved steering precision. You can count on this tyre to keep your Freelander very stable on corners even at high speeds.
2. For extensive highway drives- If you undertake extensive highway drives then you require tyres that offer a very long tread life without comprising on safety and comfort. In such a scenario, I'd say you choose out of Michelin Latitude tour HP or Pirelli Scorpion Verde. Both these tyres offer superb wet and dry grip, along with good comfort and a quiet ride quality. Michelin Latitude, although, would offer longer tread life.
3. For mild off-roading or for rough roads- If you drive over rough roads or often take your car for off-roading excursions then go for Yokohama Geolandar A/T G015. It is a very durable tyre and takes over rough roads with great ease. It also offers a long tread life.